It's really important to remember NOT to feed high numbers. That was a bounce, you have to wait for those numbers to clear. Giving more insulin won't bring it down any faster and you actually encourage more bounces to happen when you do this. Please please remember to hold the dose
no matter how high he is until he is due for an increase after 7 days. Every time you change the dose your 7 day-count starts over, so it's really important to keep it the same.
I read in another thread you're doing PMPS shots over an hour before shooting? When you feed an hour before shooting yes, his BG raises from the food but that is a false number you're now shooting. Some cats dip an hour or two before shot-time and then go back up. So if you hadn't fed Wally and tested at ACTUAL PMPS time he may have gone up enough for full dose naturally. We can't tell for sure, but it happens in many cats. Can you start shooting when you test? That way you can stall like Chris recommended when needed.
If you stick to the advice above Wally should start having more consistent good numbers.

And thank you for editing your signature/spreadsheet! Very helpful!