Ok. So you are most likely using BCP PZI rather than ProZinc. And 100U syringes should be fine.
It is probably better to post on this forum as you are wondering about the dose. Everyone here uses or has used your insulin. The protocol we put together for PZI is in my signature in blue.
So, looking at your spreadsheet. What I see is that he is getting some low numbers on 2.5 units. Yesterday, after 12 hours, he had dropped to 49. You shoot 2 units there, which was quite dangerous. We consider 50 as a watch number for a hypo. We suggest new diabetics not get shots under 200 until they have lots of data no know how their cat is likely to react. Then yesterday he also was in lower ranges and most likely bounced up to a high number this morning.
A bounce is when their body perceives a lower than normal number and "panics". It releases extra glucose. That makes the blood level bounce up - higher than normal. So we often say, after a low number and then a high for the next test, the kitty bounced. I would guess that is also what happened with some of the blue numbers you have gotten and then the highs after.
If he were my cat, I would reduce the dose, perhaps to 2 units on the higher ranges. I wouldn't shoot under 200 but would stall, waiting 20 minutes without feeding (which raises the levels) and retesting. You want a number that is rising, not still falling. A falling number would mean the insulin is still in his body and working and you don't want to add insulin to that. And you want a number at 200 or above. Then you could give the shot, but a smidge less than your previous dose (because you don't want a cycle similar to the last one when the pre shot tests was too low to shoot)
I know this sounds complicated, but if you post here regularly we can help. This is a small, friendly forum. It is busiest in the morning and evening, EST. if you have an emergency, post here and on Health as you will get more eyes.
And Welcome!